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In ion-atom collisions, several inelastic processes can take place in addition to elastic scattering.  Among these processes, excitation of target, electron capture, and ionization (the election of electrons from the target) are considered to be dominate in the energy range concerned fusion research.  There is an amount of effort to fully understand the dynamics of ion-atom collisions from both the experimental and theoretical perspectives.  As a result of these extensive experimental and theoretical investigations, most of the elastic and inelastic processes involving bound states of target and projectile ions are well described by current theories.  However, ionization remains a challenge even for the most basic processes such as proton-hydrogen system especially at low energy.  The discrepancy in ionization cross sections between two recent experiments, i.e. Shah et al. (1998) and Pieksrna et al. (1994) is as large as a factor of six.  Reasonably reliable theoretical studies of Sidky et al. (2001), Toshima (1999) and Kolakowska et al. (1999) predicted about 20% higher value than those of experiments of Shah et al. (1981,1987) at the peak of ionization cross section, and there is a considerable disagreement among theoretical cross sections at low keV energies.  The energy dependence of theoretical and experimental results is also different.  In the present work, we have aimed to provide more insight into such unresolved problems.\u003cbr /\u003e  Heavy-particle atomic collision is a complex quantum-mechanical problem.  It involves interaction of many states both from the discrete and continuum parts of the energy spectrum and also strong couplings of many reaction channels.  Obviously, the understanding of the collisional dynamics of ion-atom system would represent a considerable advance of our basic knowledge on atomic interactions, in general.  Besides, this knowledge is essential for the understanding and interpretation of a large variety of phenomena taking part in many non-equilibrium plasmas.  The importance of heavy-particle collisions in fusion research applications and the challenges for theory have motivated me to carry out this research.\u003cbr /\u003e  In the first part of my research, I studied electron emission in H+ + H(1s), He2+ + H(1s) and He+(1s) + H+ collisions at low energy (below 20 keV /amu), using the electron translation factor corrected molecular orbital close-coupling approach.  Selection of the collision partners and energy range studied here ties closely with the application in fusion plasma experiments.  Full convergence of ionization cross sections as a function of H2+ or HeH2+ molecular basis size was achieved by including up to twenty bound states, and more than three hundred continuum states.  The results obtained by our calculation are compared with the available experimental data and various theoretical models.  Excellent agreement with the recent experiments is found for the total ionization cross sections where the experimental values are available.  This study shows that for the ionization in He2+ + H(1s) and/or He+(1s) + H+ collisions, the higher-level ladder climbing processes (i.e.  excitation  via a sequence of upper levels) are dominant as compared to direct mechanism, in which the electron is liberated by one step promotion.  On the contrary, in the H+ + H(1s) collision process, H2+ is ionized directly, and the higher levels, especially 2pπu act as a temporary trap of the ionization flux.\u003cbr /\u003e  The second part of this thesis is devoted to the calculation of spectral profiles of Li2+ ions emitted in magnetically confined plasma.  In magnetic confined plasmas, Li2+ forms are populated by three kinds of mechanism;  excitation from the ground state, electron-ion recombination from Li3+ and charge exchange with neutral hydrogen and Li3+.  The nl-resolved population densities of exited Li2+ ions are calculated up to n=2O using a collisional-radiative model including the charge exchange process.  Since reliable cross sections for charge exchange processes in Li3+ + H(1s) collision are available, instead of attempting recalculations of charge transfer process, I adopt them from the recent literatures.  In the calculation, the radiative transition probabilities and wavelengths of Li2+ ions are computed by diagonalizing the Hamiltonian including interactions with the magnetic field.  This study shows that 1) spectral profiles emitted by excitation, recombination and charge exchange are quite different from each other, which is due to the different n and l-distributions of the rate coefficients of such basic atomic processes (i.e. excitation, recombination and charge exchange);  and 2) in order to interpret properly low temperature spectra, the Zeeman effect has to be accounted for, especially for ion temperature diagnostics.\u003cbr /\u003e  In summary, I have treated heavy-particle atomic collisions, which are typical in plasma, obtaining new cross sections for charge transfer, excitation and ionization at low energies.  The detailed discussions are made to collisions involving the partially or fully ionized main component of fusion plasmas (hydrogen and helium).  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  1. 020 学位論文
  2. 物理科学研究科
  3. 10 核融合科学専攻

Collision Processes of Low Charge Ions with Atoms in Fusion Plasma

https://ir.soken.ac.jp/records/502
https://ir.soken.ac.jp/records/502
170bc9d0-c6f1-4777-a4e3-5d45d093d1be
名前 / ファイル ライセンス アクション
甲674_要旨.pdf 要旨・審査要旨 / Abstract, Screening Result (479.5 kB)
甲674_本文.pdf 本文 (6.4 MB)
Item type 学位論文 / Thesis or Dissertation(1)
公開日 2010-02-22
タイトル
タイトル Collision Processes of Low Charge Ions with Atoms in Fusion Plasma
タイトル
言語 en
タイトル Collision Processes of Low Charge Ions with Atoms in Fusion Plasma
言語
言語 eng
資源タイプ
資源タイプ識別子 http://purl.org/coar/resource_type/c_46ec
資源タイプ thesis
著者名 鄒, 士陽

× 鄒, 士陽

WEKO 8672

鄒, 士陽

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フリガナ ゾウ, シヤン

× ゾウ, シヤン

WEKO 8673

ゾウ, シヤン

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著者 ZOU, Shi-Yang

× ZOU, Shi-Yang

WEKO 8674

en ZOU, Shi-Yang

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学位授与機関
学位授与機関名 総合研究大学院大学
学位名
学位名 博士(理学)
学位記番号
内容記述タイプ Other
内容記述 総研大甲第674号
研究科
値 数物科学研究科
専攻
値 10 核融合科学専攻
学位授与年月日
学位授与年月日 2003-03-24
学位授与年度
2002
要旨
内容記述タイプ Other
内容記述 Collision processes of low charged ions with neutral atomic particles at low to intermediate energies play vital roles in various fields of applied physics such as plasma physics, astrophysics, and radiation physics. In ion-atom collisions, several inelastic processes can take place in addition to elastic scattering. Among these processes, excitation of target, electron capture, and ionization (the election of electrons from the target) are considered to be dominate in the energy range concerned fusion research. There is an amount of effort to fully understand the dynamics of ion-atom collisions from both the experimental and theoretical perspectives. As a result of these extensive experimental and theoretical investigations, most of the elastic and inelastic processes involving bound states of target and projectile ions are well described by current theories. However, ionization remains a challenge even for the most basic processes such as proton-hydrogen system especially at low energy. The discrepancy in ionization cross sections between two recent experiments, i.e. Shah et al. (1998) and Pieksrna et al. (1994) is as large as a factor of six. Reasonably reliable theoretical studies of Sidky et al. (2001), Toshima (1999) and Kolakowska et al. (1999) predicted about 20% higher value than those of experiments of Shah et al. (1981,1987) at the peak of ionization cross section, and there is a considerable disagreement among theoretical cross sections at low keV energies. The energy dependence of theoretical and experimental results is also different. In the present work, we have aimed to provide more insight into such unresolved problems.<br />  Heavy-particle atomic collision is a complex quantum-mechanical problem. It involves interaction of many states both from the discrete and continuum parts of the energy spectrum and also strong couplings of many reaction channels. Obviously, the understanding of the collisional dynamics of ion-atom system would represent a considerable advance of our basic knowledge on atomic interactions, in general. Besides, this knowledge is essential for the understanding and interpretation of a large variety of phenomena taking part in many non-equilibrium plasmas. The importance of heavy-particle collisions in fusion research applications and the challenges for theory have motivated me to carry out this research.<br />  In the first part of my research, I studied electron emission in H+ + H(1s), He2+ + H(1s) and He+(1s) + H+ collisions at low energy (below 20 keV /amu), using the electron translation factor corrected molecular orbital close-coupling approach. Selection of the collision partners and energy range studied here ties closely with the application in fusion plasma experiments. Full convergence of ionization cross sections as a function of H2+ or HeH2+ molecular basis size was achieved by including up to twenty bound states, and more than three hundred continuum states. The results obtained by our calculation are compared with the available experimental data and various theoretical models. Excellent agreement with the recent experiments is found for the total ionization cross sections where the experimental values are available. This study shows that for the ionization in He2+ + H(1s) and/or He+(1s) + H+ collisions, the higher-level ladder climbing processes (i.e. excitation via a sequence of upper levels) are dominant as compared to direct mechanism, in which the electron is liberated by one step promotion. On the contrary, in the H+ + H(1s) collision process, H2+ is ionized directly, and the higher levels, especially 2pπu act as a temporary trap of the ionization flux.<br />  The second part of this thesis is devoted to the calculation of spectral profiles of Li2+ ions emitted in magnetically confined plasma. In magnetic confined plasmas, Li2+ forms are populated by three kinds of mechanism; excitation from the ground state, electron-ion recombination from Li3+ and charge exchange with neutral hydrogen and Li3+. The nl-resolved population densities of exited Li2+ ions are calculated up to n=2O using a collisional-radiative model including the charge exchange process. Since reliable cross sections for charge exchange processes in Li3+ + H(1s) collision are available, instead of attempting recalculations of charge transfer process, I adopt them from the recent literatures. In the calculation, the radiative transition probabilities and wavelengths of Li2+ ions are computed by diagonalizing the Hamiltonian including interactions with the magnetic field. This study shows that 1) spectral profiles emitted by excitation, recombination and charge exchange are quite different from each other, which is due to the different n and l-distributions of the rate coefficients of such basic atomic processes (i.e. excitation, recombination and charge exchange); and 2) in order to interpret properly low temperature spectra, the Zeeman effect has to be accounted for, especially for ion temperature diagnostics.<br />  In summary, I have treated heavy-particle atomic collisions, which are typical in plasma, obtaining new cross sections for charge transfer, excitation and ionization at low energies. The detailed discussions are made to collisions involving the partially or fully ionized main component of fusion plasmas (hydrogen and helium). Based on a detailed computation for spectral profiles of Li2+ ions, I have analyzed the spectra of hydrogen-like lithium measured from magnetic confinement fusion plasmas.
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